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Table of Content

    25 October 2014, Volume 42 Issue 10
    Materials Science & Technology
    Ye Jian-dong Wu Hua-e He Fu-po Zhang Jing
    2014, 42(10):  1-6.  doi:10.3969/j.issn.1000-565X.2014.10.001
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    Calcium phosphate cement (CPC) was modified by incorporating the lyophilized powders of plateletrich plasma (PRP) and plateletpoor plasma (PPP), and the effects of PRP or PPP on the hydration product phase, section morphology and cell response of CPC were characterized by means of XRD, SEM and cell experiments. The results show that (1) incorporating PRP or PPP does not affect the hydration products of CPC, and the final hydration product is nothing but poorly crystalline hydroxyapatite; (2) incorporating an appropriate amount of lyophilized powders of PRP or PPP into CPC greatly promotes the adhesion, proliferation and differentiation of human mesenchymal stem cells (hMSCs) on CPC; and (3) in the late stage of cell culture, incorporating a smaller amount of PRP helps to improve cell proliferation and differentiation. Therefore, it is expected that PRP and PPP can be used to improve the cell response and osteoinductivity of CPC.

    Zuo Xi Li Wen-fang Mu Song-lin
    2014, 42(10):  7-13.  doi:10.3969/j.issn.1000-565X.2014.10.002
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    In this paper,two additives including vanadate and organic were added in the mixed Ti-Zr solution ,and the effects of these additives on the behaviors of Ti-Zr conversion coating were investigated.Then,the micrographic structure and thickness of the coating were analyzed by using an optical microscope and eddy current thickness meter,respectively,and the corrosion resistance of the coating was discussed by dropping corrosion test,Tafel polarization curves and electrochemical spectroscopy(EIS).The results indicate that,with the coordination effect of vanadate and organic,Ti-Zr conversion coating can be prepared at room temperature with a time consumption of only 30s,the thickness,anti-corrosion time,corrosion current density and impedance of the coating are respectively 4,3,1/6,and 3 times that of the coating without any additives.It is thus concluded that the optical corrosion resistance of conversion coating was prepared by added the two additives simultaneously into Ti-Zr solution.

    Liu Hong Liu Zhong-wu Yin Yu-hang
    2014, 42(10):  14-19.  doi:10.3969/j.issn.1000-565X.2014.10.003
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    A kind of ceramic matrix cubic boron nitride (cBN) composites for bearing interfacial precision grinding was prepared by sintering process. The microstructure and element distribution at the interfaces were studied by scanning electron microscope and electron probe analysis. The grinding properties were tested by bearing interfacial grinder. The results show that with the increase of sintering temperature, the composition diffusion depth at the interfaces increases slowly, and the interfacial binding strength increases more rapidly than the strength of ceramic matrix. At the sintering temperature of 750 ℃, interfacial binding strength of composites matches well with the matrix strength. With the feed rate is 8 μm/r and the abrasion volume ratio is 310-370, the ceramic matrix cBN composites show good grinding performance with high sharpness and wear resistance. The wear, rupture, exfoliation of cBN and the fracture of ceramic matrix material were observed after grinding.

    Xiao Xin-yan Shi Ying-long Liu Jian-feng
    2014, 42(10):  20-24,30.  doi:10.3969/j.issn.1000-565X.2014.10.004
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    First, with tetraethoxysilane (TEOS) as precursor and methyltriethoxysilane (MTES) as modifier, hydrophobic silica nano-particles were synthesized in polyacrylate emulsion containing siloxane and fluorine (FSiPA) by means of the sol-gel method. Next, superhydrophobic coatings were fabricated by spraying the SiO2/FSiPA hybrid emulsion on clean glass substrates. Then, the authors analyzed the effects of the FSiPA emulsion dosage and the mole ratio of MTES to TEOS (M/T) on the coating performance were analyzed and explored the effect of M/T on the coating micro-morphology was explored. Finally, the formation mechanism of the hybrid coating was discussed, and the self-cleaning properties of the superhydrophobic and hydrophobic coating tilting at the same angle were also compared. The results show that, when the FSiPA emulsion content iswas 15% and the M/T iswas 5, the coating possesses good film-forming property and self-cleaning property with a water contact angle of about 154.0°, and the hydrophobic silica particles can form rough micro/nanostructure on the coating surface.

    Liu Shu-mei Feng Meng Sun Zhi-song Zhao Jian-qing Yuan Yan-chao
    2014, 42(10):  25-30.  doi:10.3969/j.issn.1000-565X.2014.10.005
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    A spiro and caged bicyclic phosphate flame retardant named as PDD-PEPA was synthesized with pentaerythritol diphosphate dichloride (PDD) and caged bicyclic phosphate 1-oxo-1-phospha-2, 6, 7–trioxabicyclo [2.2.2]-4-hydroxymethyl octane (PEPA) as reactants, and the synthesis conditions of the flame retardant, namely the dosage of triethylamine as a catalyst and the reaction time, wereare optimized. Then, the structure of PDD-PEPA was characterized by means of MS, IR and NMR, and the thermal stability and charring capacity of PDD-PEPA were investigated in N2 atmosphere through thermalgravimetric analysis. The results show that (1) when PDD- and PEPA reacts with a mole ratio of triethylamine to theoretical hydrogen chloride of 1:2 in the acetonitrile solvent at a reflux temperature for 10 h, the yield of PDD-PEPA is higher, and (2) under such conditions, the theoretical phosphorus content of the flame retardant is 21.2%, the initial decomposition temperature is 351℃, and the carbon yield is 63.6% at 650℃.

    Duan Qiang Yan Jun Zhu Guo-hui Cai Qing-wu
    2014, 42(10):  31-35,43.  doi:10.3969/j.issn.1000-565X.2014.10.006
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    In the investigation, the microstructural observation and quasistatic tension experiments of X80 pipeline steel were conducted so as to reveal the effects of the cooling rate on its quenched dual-phase microstructure formation and strain-hardening behavior. The results show that (1) a dual-phase microstructure including ferrite and bainite is obtained after X80 pipeline steel is quenched; (2) the ferrite volume fraction and the uniform elongation increase with the decrease of the cooling rate while the strength decreases; (3) when the ferrite volume fraction is not less than 5.27%, the strain-hardening exponent has a positive correlation with the uniform elongation but a negative correlation with the yield ratio; (4) when the ferrite volume fraction reaches up to 22.8%, the work-hardening rate decreases with a fast stage and then a slow stage, and the latter stagethe later stage delays the necking point; and (5) with the decrease of the cooling rate, the lath-like bainite in the quenched microstructure turns to be granular and MA phase forms, simultaneously, the strain-hardening performance of the quenched microstructure is guaranteed and the uniform plastic deformation ability is improved by means of the conversion of the dislocation strengthening to the second phase strengthening.

    Yin Xiao-chun Tang Bang Zeng Wen-bing Yang Zhi-tao Qu Jin-ping
    2014, 42(10):  36-43.  doi:10.3969/j.issn.1000-565X.2014.10.007
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    In the investigation, the structure and working principle of a vane compounder dominated by dynamic tensile deformation were introduced, and PS/HDPE melt blending experiments were conducted on the vane compounder and a commercial Brabender rotor internal mixer dominated by shear deformation. Then, the influences of the rotating speed and the mixing time on the mechanical property, rheological property and microstructure of the blends were discussed. The results show that (1) the tensile strength of the PS/HDPE blends molded by the vane compounder first increases and then keeps stable with the increases of the mixing time and the rotating speed, which is similar to those of the Brabender rotor internal mixer; (2) as compared with the Brabender rotor internal mixer, the rotating speed of the vane compounder has a smaller effect on the particle size of the dispersion phase of the blends, and the vane compounder needs a shorter time to achieve the same particle size of the dispersion phase at the same rotating speed; (3) the apparent viscosity of the blends molded by the Brabender rotor internal mixer remains unchanged with the increases of the mixing time and the rotating speed while that of the vane compounder decreases; and (4) the vane compounder shows a higher mixing efficiency and a better mixing effect in comparison with those of the Brabender rotor internal mixer.

    Li Li-feng Ren Li Liu Sa Wang Ying-jun
    2014, 42(10):  44-49,56.  doi:10.3969/j.issn.1000-565X.2014.10.008
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    A medical bacterial cellulose medium with simple and definite components waswere obtained by adding trace elements with coconut juice as the basic carbon source and the growth factor source, yeast extract as the nitrogen source and ethanol as the addition carbon source. The medium contains components with relatively stable content and can improve the fermentation rate and the yield of bacterial cellulose, and the product thickness can meet various medical requirements. Then, alkali is used to purify the fermentation product by combining SDS or ultrasound or ethanol. The results show that alkali and SDS treatment procedure has the best purification effect, and that the purified sample possesses a content of impurity nitrogen below the detection limit and a high transmittance which is close to cornea in vivo in the visible region, and it exhibits a good biocompatibility  withto L929 cells.

    Liu Ding-fu Liang Ji-zhao Ge Ming-liang
    2014, 42(10):  50-56.  doi:10.3969/j.issn.1000-565X.2014.10.009
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    In order to obtain the low-temperature expandable graphite (LTEG) by means of a low pollution method, the natural flake graphite (NFG) was oxidized in the perchloric acid solution by means of the electrochemical method. Thus, the sulfur-free LTEG of a large exfoliated volume (EV) and a low initial exfoliating temperature was prepared. Then, the influences of the current density, the electrolysis time, the mass fraction of HClO4 in electrolyte and the exfoliating temperature on the EV were discussed, and the LTEG was characterized by means of FTIR, TGA and XRD. The results show that (1) the mass fraction of HClO4 in electrolyte can be as low as 50%, which dramatically decreases in comparison with the results of chemical oxidation methods; (2) recycling the electrolyte is easy, which helps to reduce environmental pollution; (3) the EV of the LTEG reaches up to 282 mL/g and 594 mL/g respectively at the exfoliating temperatures of 200 ℃ and 950 ℃, and the LTEG is high-rate, sulfur-free and expandable at low temperatures; (4) there exists  carbonyl and carboxyl on the surface of the LTEG, and there exists ClO4- and HClO4 as intercalation compounds within the space between the graphite pieces; (5) the intensity of the characteristic diffraction peak at a 2θ of 25.76 º is very weak, and a broad peak appears at a 2θ of 9.41 º with an interlayer distance of 0.94 nm; and (6) the thermal weight loss of the LTEG occurs obviously between 60~330 ℃ with a thermal weight loss rate of about 28%, and the total thermal weight loss rate is about 35% between 60~800 ℃.

    Jia Run-ze Wang Yi-chun Zhou Fei
    2014, 42(10):  57-62.  doi:10.3969/j.issn.1000-565X.2014.10.010
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    An experiment on two prepared Fe-Co-Ni MRFs (Magneto Rheological Fluids) was conducted through a homemade device. Then, the electrical and thermal conductivities of the two MRFs wereare analyzed and compared with those of the Fe-Co-Ni magnetic powder itself. The results show that the magnetic field causes the electrical and thermal conductivities of the Fe-Co-Ni MRFs and magnetic powder to change greatly, and that, when the magnetic field intensity increases within 0~0.92T, the resistance of the Fe-Co-Ni magnetic powder decreases by two-to-three orders of magnitude with a significant increase in thermal conductivity increase which is from 4W/(m2•K) to 13.2W/(m2•K), and the thermal conductivities of the two MRFs also increase.

    Chemistry & Chemical Engineering
    Deng Yong-hong Guo Yun-qing Qiu Xue-qing Lou hong-ming
    2014, 42(10):  63-69.  doi:10.3969/j.issn.1000-565X.2014.10.011
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    In order to reveal the influence of the structure of the modified lignin GCL1-JB on its adsorption characteristics and dispersion stability, a series of GCL1-JB of different conformations were prepared by adding dioxane into the aqueous solution of GCL1-JB. Then, the dispersion stability of cement/GCL1-JB suspension and the adsorption characteristics of GCL1-JB of different conformations were determined by using a TurbiscanLab analyzer and by means of the sequential adsorption process. The results show that with the increase of the stretch conformation of GCL1-JB, the amount of GCL1-JB adsorbed on a solid surface decreases while the dispersion stability of GCL1-JB for cement particles increases. In addition, the GCL1-JB of more stretch conformation can adsorb flat  and forms a compact and smooth film, thus effectively preventing cement particles from agglomerating. This is why the dispersion stability of GCL1-JB is superior to that of sodium lignosulfonate.

    Wu Shu-bin Deng Yu-bin Liu Chao
    2014, 42(10):  70-74.  doi:10.3969/j.issn.1000-565X.2014.10.012
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    In order to deeply investigate the pyrolysis mechanism of lignin, its pyrolysis process is simulated with vanillin, vanillic alcohol and vanillic acid being selected as monomeric model compounds of lignin. In the investigation, the density functional theory is employed to analyze the dissociation sequences of chemical connection bonds, and four reaction paths, namely, Path 1 - Path 4, are designed. Both Path 1 and Path 2 generate guaiacol  but their intermediate processes are not the same, while Path 3 and Path 4 generate catechol and phenol with priority processes respectively. The results show that (1) the methyl in the side chains of the model compounds first dissociates with CH4 being released, and the dissociation sequences of the substituents on C1 depend on their ability to withdraw electrons; (2) in the pyrolysis process, it is difficult for the substituents on C1 to dissociate directly, but prior dissociation occurs instead with the help of outside factors; (3) it is possible for the target products of three kinds to be obtained in the priority sequence of catechol, phenol and guaiacol; (4) from the view of dynamics, Path 2 and Path 4 are superior to Path 1 and Path 3 in terms of dynamic progress; and (5) whenever the target products of the same kind are made,  it is always the easiest job for vanillic alcohol, and then vanillin, whereas vanillic acid is always  the most difficult matter to be dealt with.

    Long Xin-feng Wu Juan
    2014, 42(10):  75-81.  doi:10.3969/j.issn.1000-565X.2014.10.013
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    The Ca(OH)2/CaO system is a very promising thermochemical energy storage medium, and its kinetic research provides an important way ofto understanding  the reaction and energy storage/release rates of the whole energy storage system. In this paper, a thermogravimetric analysis iswas  conducted to investigate the thermal decomposition processes of Ca(OH)2 samples in pure N2 atmosphere at different heating rates. The results show that during the thermal decomposition of Ca(OH)2 samples, two weight loss processes occur at 623.15~773.15 K and 873.15~973.15 K, and the weight loss rates are close to 21% and 2%, respectively. The kinetic analysis of the thermal decomposition process through the multiple scanning indicates that the obtained apparent kinetic parameters depend on the reaction conversion rate, the heating rate and the selected model approach. Through the most probable mechanism function analysis, it is also found that the thermal decomposition kinetics model of Ca(OH)2 under experimental conditions accords well with the shrinking cylinder mechanism with surface reaction rate controlling. Besides, there exists a linear relationship between the activation energy E and the natural logarithm of the pre-exponential factor A at different heating rates.

    Yuan Teng Chen Zhuo Liu Wen-ji Zhou Xian-hong Tu Wei-ping Wang Feng
    2014, 42(10):  82-89.  doi:10.3969/j.issn.1000-565X.2014.10.014
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    The current oil/water separation membrane researches based on special wettability are seldom involved in the dynamic process of the membrane separation and the relevant quantitative calculations. In this paper, by analyzing the physical quantities of the superhydrophilic membrane separation process based on the capillary mechanics and by classifying the membrane pores of membrane materials based on special wettability as capillary pores, a mathematical model is constructed, and it is used to analyze the force distribution condition in the separation process of oilwater mixture by using the superoleophilic membrane. Then, the principle of the superhydrophilic and superoleophilic membrane in the air transforming to be superoleophobic underwater is analyzed from the perspective of surface tension, and the capillary flow rate, the capillary permeation rate, the membrane flux and the critical penetration pressure in the membrane separation process are calculated based on capillary mechanics and are validated by experiments. On this basis, the separation mechanism of superhydrophilic and underwater superoleophobic oil/water separation membrane is preliminarily discussed based on capillary mechanics.

    Yang Xiao-dong Wang Lei Lu Xin-wei Liu Rui-yuan Qu Jin-qing
    2014, 42(10):  90-94.  doi:10.3969/j.issn.1000-565X.2014.10.015
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    2-(6-hydroxynaphthalen-2-methylene) malononitrile (probe 1) was synthesized by means of the reaction of malononitrile and 6-hydroxy-2-naphthaldehyde, and the product was used as a fluorescent probe for the detection of fluoride ions. The results show that, in the detection system, the DMSO solution of probe 1 is pale yellow without fluorescence, and it immediately turns to be pink with blue-fluorescence after adding fluoride ions but shows no fluorescence after adding other anions. It is also found that probe 1 exhibits a strong selectivity and a high sensitivity to fluoride ions. According to the evaluation of the Job’s plot, the ratio of probe 1 to fluoride ions in the complex is found to be 1:1. The 1H NMR titration results confirm that the deprotonation of phenolic hydroxyl of probe 1 occurs after adding fluoride ions. The calculation results based on the Frontier molecular orbital theory indicate that, after the deprotonation of probe 1, its HOMO–LUMO energy gap increases, and the solution color and the fluorescence spectrum change dramatically.

    Gao Wen-hua Chen Ke-fu Yang Ren-dang Yang Fei
    2014, 42(10):  95-101.  doi:10.3969/j.issn.1000-565X.2014.10.016
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    The coating process is one of the core technologies forin the manufacture of reconstituted tobacco. In the investigation, three rheological additives, namely CMC, GG-50 and CGG, were respectively added into the coating to adjust the coating properties and improve the coating process. Then, the relationship between the additives and the properties of the reconstituted tobacco after coating is discussed. The results show that (1) with the increase of the rheological additive dosage, the coating viscosity and the tensile strength and the tear index of the reconstituted tobacco after coating increase while the bulk, the air permeability and the filling value of the reconstituted tobacco after coating decrease; (2), simultaneously, the release amounts of tar, total particulate matter and carbon monoxide in the main smoke also rise. The SEM analysis of reconstituted tobacco shows that when all the dosages of the three rheological additives are all 0.1%, the coating structure on the reconstituted tobacco surface is better, , the coating fills in the inside of reconstituted tobacco base-paper, and there is no fragment on the coating surface.

    Architecture & Civil Engineering
    Meng Gang Jia Jin-qing Gao Jun-cheng Ye Hao
    2014, 42(10):  102-109,116.  doi:10.3969/j.issn.1000-565X.2014.10.017
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    The crack width directly affects the durability and normal use of structures. In order to investigate the crack resistance of prestressed steel-reinforced ultra-high strength concrete beams, the flexural behaviors of thirteen specimens were tested. Then, this paper analyzes the failure mode and the development and distribution of cracks as well as the maximum crack width were analyzed, and puts forward the relationship between the integrated reinforcement index considering the reinforcement position and the moment under the serviceability limit state was investigated. Based on the existing relevant norms in China, the calculation formula of the average crack spacing and the maximum crack width are proposed, which are appropriate for prestressed steel reinforced ultra-high strength concrete beams. It is found that the calculation results accord well with the test results. In addition, when the web effect is taken into account, the webs of the tension side in a 1/2 beam height range are considered to be equivalent to the longitudinal reinforcement, which leads to the finding that  the calculation values with an integrated reinforcement index of more than 0.19 are slightly greater than the measured ones while the calculation values with an integrated reinforcement index of less than 0.19 are slightly smaller than the measured ones.

    Yang Tao Lan Wen-wu Qian Kai
    2014, 42(10):  110-116.  doi:10.3969/j.issn.1000-565X.2014.10.018
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    The local or global progressive collapse of reinforced concrete (RC) flat slab structures may occur due to the failure of load-bearing columns under the accidental loading, such as explosion and impact. In order to investigate the effect of slab reinforcement details on the progressive collapse performance of RC flat slab structures, two one-third scale RC flat slab substructure models are constructed and tested under monotonic static load in the scenario of loss of a corner column. Experimental results show that (1) continuous top slab reinforcement can effectively reduce the width of cracks on the slab; (2) as compared with the specimen with arranging discontinuous top slab reinforcement, the yield load, first peak load and ultimate bearing capacity of the substructure witharranging continuous top slab reinforcement increase respectively by 38.4%, 31.8% and 7.5%, and the progressive collapse resistance under dynamic load is significantly improved as well; and (3) the tensile membrane action in the slabs contributes significantlymake a significant contribution to the progressive collapse resistance after the working mechanism of yield lines fails.

    Ma Ming-lei Ma Ru-jin Chen Ai-rong
    2014, 42(10):  117-124.  doi:10.3969/j.issn.1000-565X.2014.10.019
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    Aiming at the growing concern over the fire risk of bridges, the fire resistance of a long-span cable-stayed bridge is analyzed by means of the performance-based method. First, different types of vehicles, namely, car, bus, van, heavy goods truck and petrol tanker, are selected as fire risk sources, and three kinds of fire scenarios on deck are designed. Next, the flame temperatures of different fire scenarios are obtained by using FDS (Fire Dynamics Simulator), and they are compared with those of the ISO834 curve. Then, the temperatures of stay cables are acquired respectively by using the FDS and the ISO834 curve, and the failure conditions of the cables are also discussed by taking into account the yield strength variation. Finally, the safety of the full bridge is assessed. The results show that (1) the flame temperatures obtained through FDS simulations are generally lower than those of the ISO834 curve, and three cables may fail in the most serious case;, and (2) that, fires have a limited influence on the overall safety performance of bridges but can weaken the using function, so it’s necessary to take effective measures to reduce the loss caused by fires.

    Chen Yu-feng Chen Wu-jun Zhao Bing
    2014, 42(10):  125-130.  doi:10.3969/j.issn.1000-565X.2014.10.020
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    In the investigation, a dumbbell-shape ETFE foil specimen is employed to conduct mono-uniaxial tensile tests, thus obtaining commonly-used mechanical parameters, namely, yield strength, yield strain, tangent modulus and secant modulus. According to the visco-elastic and plastic features of ETFE foils, the equivalent strain energy method is adopted to calculate the equivalent elastic modulus of ETFE foils. It is found that the calculated equivalent elastic modulus falls in between the tangent modulus and the secant elastic modulus. Then, a set-up is developed particularly for the biaxial test of ETFE foils and is used to perform a series of corresponding tests, and the decoupled biaxial elastic modulus is formulated according to the orthotropic elastic film engineering theory. Based on the stress-strain curve of the biaxial tensile test of ETFE foils, the coupled modulus of a 250mm ETFE foil is found to be 1163MPa at the bilateral stress ratio of 1:1. Based on the orthotropic theory, the decoupled modulus of the ETFE foil is found to be 814.2MPa, which is close to the equivalent elastic modulus obtained through the uniaxial tensile test.

    Guo Hao-xu Li Yan Deng Meng-ren Zhao Fei-xiang
    2014, 42(10):  131-137.  doi:10.3969/j.issn.1000-565X.2014.10.021
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    The balance of the commercial flow distribution is known as the key link in the design of commercial buildings, and the commercial flow distribution is predicted based on the previous experience of some experts, which inevitably proves  to be become subjective or obsolete to some extent. The development of space syntax helps to obtain a more accurate predication of pedestrian flow distribution. This paper takes two typical shopping malls in Guangzhou as prototypes to conduct simulations in different spatial organization patterns by using the Depthmap and SPSS softwares. The results indicate that (1) under the condition of the balanced distributions of entrance and vertical transportation, the method combining integration with tenants can be used to predict the pedestrian flow distribution more effectively; (2) the space form of concise organization and relative symmetry helps to realize a balanced pedestrian flow distribution; and (3) when the C spatial organization is poor, reasonable tenants combination helps to improve sharing to a certain degree.

    Liu Pei-jie Zhao Yue-zhe Wu Shuo-xian
    2014, 42(10):  138-144.  doi:10.3969/j.issn.1000-565X.2014.10.022
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    The newly-built elevated stations of high-speed railway in China have oversize waiting halls, and intensive researches on the architectural acoustics of such oversize volume room are insufficient. In this paper, by taking a waiting hall as an example, room acoustic parameters are analyzed by means of in-situ measurement and computer simulation techniques. The results show that (1) the reverberation time (RT) of the waiting hall are rather long, and the average reverberation time in medium frequency is 9.21s, which is longer than those in low and high frequencies; (2) in the waiting hall within 500~1kHz, the speech transmission index (STI) is highly relevant to the early decay time (EDT) but is lowly relevant to the RT; (3) enlarging the sound absorption area of surfaces can significantly improve the room acoustic parameters; (4) A weighted sound pressure level is highly relevant to the logarithm value of the source-receiver distance while the RT within 500~1kHz is irrelevant to the source-receiver distance; and (5) within a certain source-receiver distance, the EDT within 500~1kHz, the speech articulation within 500~1kHz and the STI are highly relevant to the distance. Besides, the distances between the distributed loudspeaker system in the waiting hall and the passengers should be carefully designed so as to meet the requirement of speech articulation.

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